Polariton transport in 2D semiconductors:Phonon- mediated transitions between ballistic,superdiffusive, and exciton-limited regimes
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American Association for the Advancement of Science
Abstract
Exciton transport in 2D semiconductors holds promise for room temperature, ultracompact optoelectronic devices, but it is limited by short propagation distances. Hybridization of excitons with cavity photons to form exciton-polaritons can enhance the propagation by orders of magnitude, enabling a coherent, ballistic transport. However, a microscopic understanding of the role of phonons is still lacking, particularly regarding their influence on the crossover from the ballistic to the diffusive polariton transport regime. Here, we investigate the spatiotemporal polariton dynamics in MoSe2 monolayers at moderate to high temperatures, explicitly including the phonon-mediated coupling to the intervalley exciton reservoir. We identify three distinct transport regimes: (i) an initial subpicosecond ballistic-like regime characterized by a phonon-induced velocity renormalization, (ii) a transient, few-picosecond superdiffusive regime characterized by strongly enhanced diffusion, and (iii) a slower, exciton-limited diffusion following thermalization. The gained microscopic insights will trigger and guide future experimental studies on the phonon-mediated polariton transport in atomically thin semiconductors.
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Philipps-Universität Marburg
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Except where otherwise noted, this item's license is described as Attribution 4.0 International